Electronic and Vibrational Coherence in Photosynthetic and Model Systems
Ultrafast optical response and excitation energy dynamics in light harvesting pigment-protein complexes and in a few model systems have been studied both experimentally and theoretically. Femtosecond light pulses were employed to excite the system and monitor the subsequent time evolution of the transient absorption kinetics and anisotropy. A new form of pump-probe technique was developed for perf